Journal article

Tuning valence tautomerism in a family of dinuclear cobalt complexes incorporating a conjugated bridging bis(dioxolene) ligand with weak communication

TE Fischer, JT Janetzki, FZ M. Zahir, RW Gable, AA Starikova, C Boskovic

Dalton Transactions | ROYAL SOC CHEMISTRY | Published : 2024

Abstract

Valence tautomerism (VT) involves the stimulated reversible intramolecular electron transfer between a redox-active metal and ligand. Dinuclear cobalt complexes bridged by bis(dioxolene) ligands can undergo thermally-induced VT with access to {CoIII-cat-cat-CoIII}, {CoIII-cat-SQ-CoII} and {CoII-SQ-SQ-CoII} states (cat2− = catecholate, SQ˙− = semiquinonate, CoIII refers to low spin CoIII, CoII refers to high spin CoII). The resulting potential for two-step VT interconversions offers increased functionality over mononuclear examples. In this study, the bis(dioxolene) ligand 3,3′,4,4′-tetrahydroxy-5,5′-dimethoxy-benzaldazine (thMH4) was paired with Mentpa (tpa = tris(2-pyridylmethyl)amine, n = ..

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University of Melbourne Researchers

Grants

Awarded by Australian Government


Funding Acknowledgements

We would like to thank the Australian Research Council for financial support (DP220100398) and an equipment grant (LE210100009). T. E. F. thanks the University of Melbourne for a Dr Jim Desmarchelier Scholarship. J. T. J. acknowledges support from the Australian Government for a Research Training Stipend. A. A. S. thanks the Ministry of Science and Higher Education of the Russian Federation (State assignment in the field of scientific activity, project no. FENW-2023-0017). This work was performed, in part, at the Trace Analysis for Chemical, Earth and Environmental Sciences (TrACEES) Platform at the University of Melbourne. This research was undertaken, in part, using the MX1 and MX2 beamlines at the Australian Synchrotron, part of ANSTO, Victoria, Australia and made use of the Australian Cancer Research Foundation (ACRF) detector (for MX2). We are grateful to Dr Gemma Gransbury for her invaluable feedback and discussions, and for providing Fig. S1 dagger/Fig. 6.